im sure you could, but you would need to be like a genius because i have never seen a wireless controller that has the mem. card slots.
however, i do alot of work with remote control cars, and i do alot of mods that involve, like on 1 of my cars, i made the hood electronicly pop up, and what i did was mount the motor and everything, and then take apart a zip zap and mount that reciever in my car, and then the transmitter in my remote, and used two different crystals, or frequencys, and as simple as it seems, the way i just said it, it did work

however it was not that easy to do. lol
but i would have to say in conclusion, either use the cords with the s controller if you like the feel better, and need the mem. card slots, or if you want it wiresless just use the logitec.
ph34r